Open Access

Development of Adaptable Phase Change Material Composites for Advanced Passive Cooling of Processors

Gayathri Amutha Senthil Kumar, gayathriamuthas@gmail.com
Department of Computer Science and Engineering, K. S. Rangasamy College of Technology, Tiruchengode, TN, India
Mothilragav Manimaran, mothilragavmanimaran@gmail.com
Department of Computer Science and Engineering, K. S. Rangasamy College of Technology, Tiruchengode, TN, India
Revathi Ravichandran, revathiravichandran@gmail.com
Department of Computer Science and Engineering, K. S. Rangasamy College of Technology, Tiruchengode, TN, India
Suganthi Ganesan, suganthiganesan@gmail.com
Department of Physics, Government Engineering College, Dharmapuri, TN, India
Malarvizhi Muthubalasubramanian malarinresearch@gmail.com
Department of Physics, K. S. Rangasamy College of Technology, Tiruchengode, TN, India
Author Profile



J. Environ. Nanotechnol., Volume 15, No 1 (March 2026) pp. 469-477

https://doi.org/10.13074/jent.2026.03.2612058

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Abstract

Modern processors and data-centre modules often experience localized thermal spikes due to rapidly fluctuating computational loads, which can negatively affect device reliability, efficiency, and operational stability. Conventional cooling approaches, including air-based active cooling and conventional phase change materials (PCMs), face limitations such as low thermal conductivity, leakage during phase transition, and bulky packaging structures. In this work, a flexible PCM nanocomposite sheet was developed using paraffin wax as the base PCM reinforced with bio-carbon derived from agricultural waste, bentonite nanoclay, and cellulose fibres. The composite was fabricated using a controlled hot-press method to produce thin, adaptable PCM sheets suitable for direct processor surface integration. The hybrid filler system improves heat transfer pathways while suppressing leakage and enhancing mechanical stability. X-ray diffraction analysis confirmed the preservation of the crystalline structure of paraffin within the composite matrix. Differential scanning calorimetry showed a melting temperature of approximately 62.8 ℃ and a crystallization temperature near 59.1 ℃, indicating stable phase-change behavior. Thermal conductivity measurements increased from about 0.25 W m-1 K-1 for pure paraffin to a maximum of 0.95 W m-1 K-1 in the optimized composite. Field emission scanning electron microscopy observations revealed uniform filler dispersion and an interconnected microstructure that enhances thermal transport. The developed sustainable PCM composite demonstrates promising potential for passive cooling of processors and advanced electronic thermal management systems.

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Reference


An, Z., Perspective on nanoheat generation and dissipation in semiconductor devices, Appl. Phy. Lett., 127(19), 190501(2025).

https://doi.org/10.1063/5.0293553

Arshad, A., Faraji, H., Mark, J. and Yan, Y., A numerical study of HNCPCM filled metal-foam strips based heat sink for passive cooling, Intersoc. Conf. Therm. Thermomech. Phenomena Electron. Syst., (2021).

https://doi.org/10.1109/ITherm51669.2021.9503194

Balasundaram, P. and N. Sivaram, Sustainable thermal energy management for electronic devices: A study on paraffin wax, biochar, and aluminium composite phase change materials, J. Energy Storage, 132, 117686(2025).

https://doi.org/10.1016/j.est.2025.117686

Chen, Y., Tian, C., Tu, Y., Zhen, Z., Wu, Y., Wang, D., Jiang, M., Yue, Z., Lei, W. and Yan, W., Paraffin/graphite/boron nitride composite as a novel phase change material for rapid heat absorption in battery thermal management technology, Int. J. Heat Mass Transf., 235, 126214(2024).

https://doi.org/10.1016/j.ijheatmasstransfer.2024.126214

Elliott, J. W., Lebon, M. T. and Robinson, A. J., Optimising integrated heat spreaders with distributed heat transfer coefficients: A case study for CPU cooling, Case Stud.Therm. Eng., 38, 102354(2022).

https://doi.org/10.1016/j.csite.2022.102354

Ganatra, Y., Ruiz, J., John, A. H. and Amy, M., Experimental investigation of Phase Change Materials for thermal management of handheld devices, Int. J. Therm. Sci., 129, 358-364(2018).

https://doi.org/10.1016/j.ijthermalsci.2018.03.012

Hua, W., Zhang, L. and Zhang, X., Research on passive cooling of electronic chips based on PCM: A review, J. Mol. Liq., 340, 117183(2021).

https://doi.org/10.1016/j.molliq.2021.117183

Janumala, E., Murali, G., Reddi, V. B. and Chinnasamy, S., Investigations on a novel composite phase change material comprising paraffin wax and CQD for thermal conductivity enhancement, Therm. Sci., 27(6 Part B), 4747-4755(2023).

https://doi.org/10.2298/TSCI220911217J

Kasitz, J., Ghufran, M. and Huitink, D., Enhanced Passive Cooling in Thermal Interface Materials via Encapsulated Phase Change Material Additives, Int. Electron. Packaging Tech. Conf. Exhibi., 8, 141296(2024).

https://doi.org/10.1115/IPACK2024-141296

Kim, S., Kim, H., King, W. P. and Nenad, M., Gaussian process optimization of phase change material heat sink design, Num. Heat Trans. Part B: Fundament., 85(12), 1767-1785(2023).

https://doi.org/10.1080/10407790.2023.2273513

Kumar, N., Gupta, S. K. and Sharma, V. K., Application of phase change material for thermal energy storage: An overview of recent advances, Mater. Today: Proce., 44, 368-375(2021).

https://doi.org/10.1016/j.matpr.2020.09.745

Li, Z. R., Hu, N. and Fan, L. W., Nanocomposite phase change materials for high-performance thermal energy storage: A critical review, Energy Storage Mater., 55, 727-753(2023).

https://doi.org/10.1016/j.ensm.2022.12.037

Lin, Y., Jia, Y., Alva, G. and Fang, G., Review on thermal conductivity enhancement, thermal properties and applications of phase change materials in thermal energy storage, Renew. Sustain. energy Rev., 2018. 82(3), 2730-2742(2018).

https://doi.org/10.1016/j.rser.2017.10.002

Liu, L., Tang, Y., Di, S. and Fang, G., Thermal conductivity enhancement of phase change materials for thermal energy storage: a review, Renew. sustain. energy Rev., 62, 305-317(2016).

https://doi.org/10.1016/j.rser.2016.04.057

Navaux, P. O. A., Lorenzon, A. and da Silva Serpa, M., Challenges in high-performance computing, J. Brazil. Comp. Soc., 29(1), 51-62(2023).

https://doi.org/10.5753/jbcs.2023.2219

Omi, M. N. A., Optimization of Thermal Performance by Enhancing Natural Convection of Diverse Configurations of Fin Heat Sink Filled With Nano‐Enhanced Phase Change Materials: A Numerical Study, Heat Trans., 54(2), 1267-1280(2024).

https://doi.org/10.1002/htj.23230

Radouane, N., A comprehensive review of composite phase change materials (cPCMs) for thermal management applications, including manufacturing processes, performance, and applications, Energies, 15(21), 8271(2022).

https://doi.org/10.3390/en15218271

Rubel, R. I., Akram, M. W., Md, M. A., Nusrat, A., Raju, A. and Bari, M. A. A., Phase change materials in high heat storage application: A review, Arab. J. Sci. Eng., 49(11), 14533-14551(2024).

https://doi.org/10.1007/s13369-024-09519-z

Wang, J. X., Jian, Q., Ni, W., He, Z., Cao, X., Liu, F. and Hao, G., A scalable micro-encapsulated phase change material and liquid metal integrated composite for sustainable data center cooling, Renew. Energy, 213, 75-85(2023).

https://doi.org/10.1016/j.renene.2023.05.106

Yang, L., Jin, X., Yuan, Z. and Kai, D., Recent development on heat transfer and various applications of phase-change materials, J. Clean. prod., 287, 124432(2021).

https://doi.org/10.1016/j.jclepro.2020.124432

Zacharias, A., Baby, R., Maria, H. J. and Sabu, T., Preparation, characterization, and selection of nano-assisted phase change materials for thermal management and storage applications, Renew. Sustain. Energy Rev., 210, 115195(2025).

https://doi.org/10.1016/j.rser.2024.115195

Zheng, X., Liu, H., Lv, H., Xiao, Y., Lin, J., Lei, H., Hu, J., Algadi, H. and Li. X., Research Progress of Phase Change Materials for Thermal Management in Electronic Components, Adv. Mater. Interf., 12(18), e00573(2025).

https://doi.org/10.1002/admi.202500573

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