Open Access

Influence of Zinc Oxide Nanoparticles on the Properties of Banyan Fiber/Epoxy Composites for Biomedical Applications

M. K. Muniyasamy, munishcivilian1@gmail.com
Department of Civil Engineering, Saveetha School of Engineering, Saveetha Institute of Medical and Technical Sciences, Chennai, TN, India
M. Dinesh Kumar, daviddinesh2009@gmail.com
Department of Civil Engineering, Saveetha School of Engineering, Saveetha Institute of Medical and Technical Sciences, Chennai, TN, India
Basanth Babu K. Mohanram, bbbasanthbabu@gmail.com
Department of Civil Engineering, Ultra College of Engineering and Technology, Madurai, TN, India
ORCID
K. Ramesh, kanagavelramesh@gmail.com
Department of Civil Engineering, PSNA College of Engineering and Technology, Dindigul, TN, India
R. Muraliraja, muralimechraja@gmail.com
Department of Mechanical Engineering, Vels Institute of Science, Technology and Advanced Studies, Chennai, TN, India
A. Geetha Selvarani drgeethaselvarani@veltech.edu.in
Department of Civil Engineering, Vel Tech Rangarajan Dr. Sagunthala R&D Institute of Science and Technology, Chennai, TN, India



J. Environ. Nanotechnol., Volume 14, No 3 (September 2025) pp. 150-162

https://doi.org/10.13074/jent.2025.09.2521568

PDF


Abstract

This study examines the impact of zinc oxide nano particles (n-ZnO) on the mechanical, water absorption (WA) and morphological characteristics of banyan fibre (BF)-reinforced epoxy composite intended of the biomedical uses. The composites were prepared by hand layup procedure with varied weight percentages of n-ZnO (2%, 4%, and 6%) and BF concentrations (6%, 12%, and 18%). The study shows that the incorporation of up to 4 wt% n-ZnO increases tensile strength by 58.97%, achieving its maximum at this concentration. The flexural strength increases by 30.50% with 4 wt% n-ZnO, whilst the impact strength attains its maximum increase of 59.57% with 6 wt% n-ZnO. Water absorption measures exhibit a decline with higher n-ZnO content and prolonged exposure duration, indicating improved water resistance. The uniform distribution of n-ZnO, confirmed by scanning electron microscopy, causes improved water resistance and mechanical properties. Response surface methodology and Taguchi optimization evaluations provide additional evidence for the experimental findings and demonstrate that n-ZnO can enhance natural fiber-reinforced composites. This work illustrates that n-ZnO serves as an efficient filler to enhance mechanical properties and moister resistance in eco-friendly composite materials.

Full Text

Reference


Arunachalam, S. J., Saravanan, R., Sathish, T. and Parthiban, A., Comprehensive insights on mechanical properties of natural-synthetic fibres with nano-graphene composite, Interact., 245(1) 82 (2024).

https://doi.org/10.1007/S10751-024-01921-1

Ashok, K. G., Kalaichelvan, K. and Damodaran, A., Effect of Nano Fillers on Mechanical Properties of Luffa Fiber Epoxy Composites, J. Nat. Fibers, 19(4), 1472–1489 (2022).

https://doi.org/10.1080/15440478.2020.1779898

Baladivakar, S., Starvin, M. S. and Raj, J. B., Performance Evaluation of Natural Composites Made from Banyan and Cotton Fibers for Sustainable Thermal Insulation Applications, J. Nat. Fibers, 20(1) 2123881 (2023).

https://doi.org/10.1080/15440478.2022.2123881

Blessymol, B., Kalaiselvi, V., Yasotha, P. and Gopi, S., Comparative Study of Chemically and Green Synthesized Titanium Dioxide Nanoparticles using Leucas aspera Leaf Extract, J. Environ. Nanotechnol., 12(3), 10-13(2023).

https://doi.org/10.13074/jent.2023.09.233471

Prabhakar C. G., Reddy, M. S., Rajendrachari, S., Mahale, R. S., Mahesh, V. and Pandith, A., The Behavior of Banyan (B)/Banana (Ba) Fibers Reinforced Hybrid Composites Influenced by Chemical Treatment on Tensile, Bending and Water Absorption Behavior: An Experimental and FEA Investigation, J. Compos. Sci., 8(1), 31 (2024).

https://doi.org/10.3390/jcs8010031

Gaddala, B., Devi, K. V, Balakrishnan, V., Sundramurthy, V. P., Hariprabhu, M., Mayakannan, S., Kadaikunnan, S. and Khaled, J. M., Evaluation of detoxification performance of Pithecellobium dulce seed pod powder upon acid treatment: removal of reactive red 195-A dye and kinetic analysis, Z. Phys. Chem., 239(6), 885–910 (2024).

https://doi.org/10.1515/zpch-2024-0879

Ganapathy, T., Sathiskumar, R., Sanjay, M. R., Senthamaraikannan, P., Saravanakumar, S. S., Parameswaranpillai, J. and Siengchin, S., Effect of Graphene Powder on Banyan Aerial Root Fibers Reinforced Epoxy Composites, J. Nat. Fibers, 18(7), 1029–1036 (2021).

https://doi.org/10.1080/15440478.2019.1675219

Gul, W., Shah, S. R. A., Khan, A. and Pruncu, C. I., Characterization of zinc oxide-urea formaldehyde nano resin and its impact on the physical performance of medium-density fiberboard, Polym., 13(3), 371 (2021).

https://doi.org/10.3390/polym13030371

Sachin, H. S., Krishnaveni, K., Karthick, K., Chinnarasu, K., Prasad, H. V. P., Tonk, A. and Mayakannan, S., Experimental Study on the Mechanical Properties of Hybrid Areca and Abaca Fiber Reinforced Polymer Composites, J. Environ. Nanotechnol., 13(4), 92–101 (2024).

https://doi.org/10.13074/jent.2024.12.244977

Hariharan, G., Krishnamachary, P. C., Binoj, J. S. and Mansingh, B. B., Influence of SiC Nanoparticles Reinforcement in Areca/Tamarind Hybrid Biopolymer Composites: Thermo-mechanical, Tribological and Morphological Features, J. Bionic Eng., 20(4), 1723–1736 (2023).

https://doi.org/10.1007/s42235-023-00341-1

Jenish, I., Sahayaraj, A. F., Suresh, V., Mani, R. J., Appadurai, M., Irudaya, R. E. F., Nasif, O., Alfarraj, S. and Kumaravel, A. K., Analysis of the Hybrid of Mudar/Snake Grass Fiber-Reinforced Epoxy with Nano-Silica Filler Composite for Structural Application, Adv. Mater. Sci. Eng., 2022(1) 7805146 (2022).

https://doi.org/10.1155/2022/7805146

Jothi, A., S., Saravanan, R., Sathish, T., Haider, S. and Giri, J., Investigation of chemically treated jute/kenaf/glass fiber with TiO2 nano-filler for tensile and impact characteristics, AIP Adv., 14(4), 045133 (2024).

https://doi.org/10.1063/5.0206141

Jotiram, G. A., Palai, B. K., Bhattacharya, S., Aravinth, S., Gnanakumar, G., Subbiah, R. and Chandrakasu, M., Investigating mechanical strength of a natural fibre polymer composite using SiO2 nano-filler, Mater. Today Proc., 56, 1522–1526 (2022).

https://doi.org/10.1016/j.matpr.2022.01.176

Kovačević, Z., Pilipović, A., Meheš, M. and Bischof, S., Zero Waste Concept in Production of PLA Biocomposites Reinforced with Fibers Derived from Wild Plant (Spartium junceum L.) and Energy Crop (Sida hermaphrodita (L.) Rusby), Polym., 17(2), 235 (2025).

https://doi.org/10.3390/polym17020235

Kumar, K. P., Lokeshwar, G., Reddy, C. U. K., Shetty, N., Shahabaz, S. M. and Nargis, T., Experimental investigation of mechanical properties and morphology of ramie, bamboo, and ramie-bamboo hybrid composites with silicon carbide and alumina nano-fillers, Mater. Res. Express, 12(2) 025306 (2025).

https://doi.org/10.1088/2053-1591/adb2e3

Kumar, S., Gangil, B., Ranakoti, L., Bhandari, P., Gupta, D. and Gupta, M. K., An Investigation on Mechanical and Sliding Wear Properties of Titanium Oxide-Basalt Fiber-Based Hybrid PLA Composites Using Gray-Taguchi Approach, J. Inst. Eng. India. Ser. D, 105(3), 1515–1525 (2024).

https://doi.org/10.1007/s40033-023-00587-3

Lakshmaiya, N., Chukka, N. D. K. R., Kaliappan, S., Balaji, V., Ross, N. S. and Maranan, R., An integrated Artificial neural network technique to optimize the various parameters of Pineapple/SiO2/epoxy-based nanocomposites under NaOH treatment, Results Eng., 26, 104737 (2025).

https://doi.org/10.1016/j.rineng.2025.104737

Mayakannan, S., Raj, J. B., Raja, V. L. and Nagaraj, M., Effectiveness of silicon nanoparticles on the mechanical, wear, and physical characteristics of PALF/sisal fiber–based polymer hybrid nanocomposites, Biomass Convers. Biorefin., 13(14), 13291–13305 (2023).

https://doi.org/10.1007/s13399-023-04654-3

Meravi, M. K. and Panchore, V., Tribological and mechanical characteristics of glass/flax fiber-n-ZnO reinforced epoxy hybrid composite, Colloid Polym. Sci., 303(3), 411–426 (2024).

https://doi.org/10.1007/s00396-024-05356-6

Padma, R. A., Vemula, A. M., Prakash, B. M., Kumar, P. S., Murali, K. V. and Ramulu, J. P., Effect of Ceramic Nano Fillers in Jute Fibre Composites, Adv. Mater. Sci. Eng., 2022(1), 3057829 (2022).

https://doi.org/10.1155/2022/3057829

Prabhakar, C. G., Anand, B. K., Kataraki, P. S. and Reddy, S., A review on natural fibers and mechanical properties of banyan and banana fibers composites, Mater. Today Proc., 54, 348–358 (2022).

https://doi.org/10.1016/j.matpr.2021.09.300

Raja, T. and Anand, P., Investigations on Dynamic Mechanical Analysis and Crystalline Effect of Neem/Banyan Fiber-Reinforced Hybrid Polymer Composite, J. Test. Eval., 50(1) 479-489 (2022).

https://doi.org/10.1520/JTE20200580

Rajesh, M. M. A., Bensam, R. J., Beschi, S. S. L. and Raja, V. L., Influence of silica and alumina nanoparticles on the wear and mechanical behavior of Indian almond fiber reinforced natural composites, J. Text. Inst., 111(10), 1-10(2024).

https://doi.org/10.1080/00405000.2024.2420382

Rana, P. and Chopra, S., Extraction and Characterization of Inherently Antimicrobial Fibres from Aerial Roots of Banyan Tree, J. Nat. Fibers, 19(13), 6196–6213 (2022).

https://doi.org/10.1080/15440478.2021.1905586

Baskar, S., Subbiah, G., G, P. P., J, G., Kumar, M., K, K. P. and Kaliappan, N., Development and characterization of an epoxy matrix composite reinforced with Al2O3 embedded banyan fibers for secondary structural applications, Results Eng., 26, 105587 (2025).

https://doi.org/10.1016/j.rineng.2025.105587

Sathish, T., Saravanan, R., Arunachalam, S. J. and Parthiban, A., Flexural properties of jute/kenaf/glass fibre reinforced nano-composite, Interact., 245(1), 127 (2024).

https://doi.org/10.1007/s10751-024-01973-3

Senniangiri, N., Gokulkannan, S., Kumar, S. D. and Gokul, S., Enhancing Mechanical, Moisture Resistance, and Fire-retardant Properties of Nelumbo nucifera Fiber/Epoxy Nanocomposites with Zinc Oxide Nanoparticles, J. Environ. Nanotechnol., 14(1), 253–265 (2025).

https://doi.org/10.13074/jent.2025.03.2511215

Sumesh, K. R., Saikrishnan, G., Pandiyan, P., Prabhu, L., Gokulkumar, S., Priya, A. K., Spatenka, P. and Krishna, S., The influence of different parameters in tribological characteristics of pineapple/sisal/TiO2 filler incorporation, J. Ind. Text., 51(5_suppl), 8626S-8644S (2022).

https://doi.org/10.1177/15280837211022614

Velmurugan, D., Jayakumar, J., Bovas, H. B. A. and Raj, J. B., Experimental Investigation on the Mechanical Properties of Hybrid Composites Made with Banyan and Peepal Fibers, J. Nat. Fibers, 19(16), 14183–14194 (2022).

https://doi.org/10.1080/15440478.2022.2117260

Powered by

Powered by OJS